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Moss redshirted at Iowa before getting on the floor as a redshirt freshman in 2016-17, when the Hawkeyes went 19-15 overall (10-8 Big Ten) under head coach Fran McCaffery and reached the NIT.

In that 2016-17 season at Iowa, Moss played 34 games and made 28 starts, averaging 6.5 points, 1.6 rebounds, 0.9 assists, 0.6 steals, and 0.4 blocks in 17.1 minutes per game while shooting 41.2% from the field, 35.8% from three, and 74.2% at the line.

Moss took on a bigger role as a sophomore in 2017-18, starting all 33 games for a 14-19 Iowa team (4-14 Big Ten) and producing 11.1 points, 2.2 rebounds, and 1.9 assists per game in 24.2 minutes, with a shooting line of 42.0% from the field, 44.4% from three, and 87.9% on free throws.

His 2017-18 campaign included a signature scoring burst on February 21, 2018 against Minnesota, when he set his career-high with 32 points in an 86-82 loss, highlighted by 19 points in the final 1:36 and a 19-point run in 96 seconds.

As a junior in 2018-19, Moss again started every game (35 starts in 35 appearances) for Iowa as the Hawkeyes finished 23-12 overall (10-10 Big Ten) and reached the NCAA Tournament, and he averaged 9.2 points, 2.9 rebounds, 1.8 assists, 0.9 steals, and 0.2 blocks in 24.1 minutes per game while shooting 39.9% from the field, 42.1% from three, and 79.1% at the foul line.

In 2018-19, he was Iowa’s co-winner of the team’s Most Improved Player award, ranked fourth in the Big Ten in three-point percentage (42.1%), recorded double-doubles of 12 points and 10 rebounds against Nebraska (with five assists) and again against Maryland, and had a 21-point game versus Illinois that featured a career-high six assists with zero turnovers while going 5-for-6 from three.

Moss closed his Iowa career with NCAA Tournament games against Cincinnati (5 points in 23 minutes in a 79-72 win) and Tennessee (16 points, 5 rebounds, and 2 steals in 29 minutes in an 83-77 overtime loss), and he finished his three playing seasons at Iowa with 906 career points before transferring as a graduate to Kansas for 2019-20.

At Kansas in 2019-20, Moss played 30 games with nine starts for a Jayhawks team coached by Bill Self that went 28-3 overall (17-1 Big 12) and won the Big 12 regular-season title before the Big 12 Tournament and NCAA Tournament were canceled, and he averaged 7.9 points, 2.3 rebounds, 0.6 assists, and 0.5 steals in 24.6 minutes per game while shooting 38.7% from the field, 34.8% from three, and 91.2% at the line.

His Kansas season included a season-high 21 points versus UNC Greensboro on November 8, 2019 with 5-for-6 three-point shooting, a 20-point game at Oklahoma on January 14, 2020 in his first KU start while hitting 6-of-11 from deep and playing a career-high 38 minutes, his 1,000th career point coming against Baylor on January 11, 2020, Big 12 Newcomer of the Week honors on January 20, 2020, and he ended his NCAA career with 1,144 total points across 132 games for Iowa and Kansas combined.